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Visualizing Hidden Ultrafast Processes in Individual Molecules by Single-Pulse Coherent Control

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Release time:2018-11-02
Journal:J. Am. Chem. Soc.
Abstract:Coherent control of single quantum systems in complex environments has great potential to manipulate and understand photoinduced chemical and biological processes on a molecular level. However, heterogeneous environments usually impede full control and complicate interpretation. Here, we demonstrate photoluminescence-detected ultrafast phase-only coherent control on single organic molecules in a disordered matrix at room temperature. Combined with a multiparameter quantum dynamics identification
Co-author:R. Hildner*, U. Scherf, C.-C. Shu#*(通讯作者), K. Wilma#
Indexed by:Unit Twenty Basic Research
Discipline:化学
Document Type:J
Volume:140
Page Number:15329？15335
Translation or Not:no
Date of Publication:2018-11-22

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